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That is a very beautiful part of the Hill Country. I would suggest taking Highway 16 north out of S.A. through Bandera into Medina. Then 337 west from Medina to Vanderpool, which is another very beautiful road. Then from Vanderpool 187 north to 39 east, until Ingram where you could take 27 south/east to Kerrville, from there taking highway 16 north to Fredericksburg.
I've done most roads out in that area and I'd have to say 337 and 16 (especially between Bandera and Fredericksburg) are two of the most beautiful. Well, have fun!
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